Redox Cycling at an Array of Interdigitated Bipolar Electrodes for Enhanced Sensitivity in Biosensing**
نویسندگان
چکیده
An array of many bipolar electrodes (BPEs) can be controlled by a single pair driving yet allows for multiplexed analysis individual biomarkers or cells at once. A wide range electrochemical sensors have been devised, which operate under battery power and produce visible signals (e. g., luminescent, electrochromic) appropriate smartphone naked eye readout. These features BPEs are advantageous in the context clinical environmental sensing applications point need. However, sensitivity is poor comparison to direct measurement current an electrode, therefore, enhancement obtained active area research. Here, we describe signal amplification redox cycling accomplished interdigitation each BPE with shared electrode. We evaluate interelectrode spacing 35 m 5 m, over limit detection decreased order magnitude. Each interdigitated (IDBPE) has independent, reproducible, linear response reversible electroactive analyte. Therefore, this universal strategy spatially resolved point-of-need applications.
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ژورنال
عنوان ژورنال: ChemElectroChem
سال: 2021
ISSN: ['2196-0216']
DOI: https://doi.org/10.1002/celc.202100523